Cavity buildup dispersion spectroscopy

نویسندگان

چکیده

Abstract Measurements of ultrahigh-fidelity absorption spectra can help validate quantum theory, engineer ultracold chemistry, and remotely sense atmospheres. Recent achievements in cavity-enhanced spectroscopy using either frequency-based dispersion or time-based approaches have set new records for accuracy with uncertainties at the sub-per-mil level. However, laser scanning susceptibility to nonlinearities limits their ultimate performance. Here we present cavity buildup (CBDS), probing CO molecule as an example, which dispersive frequency shift a resonance is encoded cavity’s transient response phase-locked non-resonant excitation. Beating between optical frequencies during exactly localizes detuning from mode center, thus enables single-shot measurements. CBDS yield limited by chosen standard measurement duration currently 50 times less susceptible detection nonlinearity compared intensity-based methods. Moreover, significantly faster than previous The generality shows promise improving fundamental research into variety light–matter interactions.

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ژورنال

عنوان ژورنال: Communications physics

سال: 2021

ISSN: ['2399-3650']

DOI: https://doi.org/10.1038/s42005-021-00517-3